Time-resolved degenerate four-wave mixing in thin films of C60 and C70 using femtosecond optical pulses

M. J. Rosker; H. O. Marcy; Tallis Y. Chang; J. T. Khoury; K. Hansen; R. L. Whetten

doi:10.1016/0009-2614(92)85715-M

Time-resolved degenerate four-wave mixing in thin films of C₆₀ and C₇₀ using femtosecond optical pulses

M. J. Rosker
, H. O. Marcy
, Tallis Y. Chang
, J. T. Khoury
, K. Hansen
, R. L. Whetten

Research output: Contribution to journal › Article › peer-review

86 Scopus citations

Abstract

Thin films of pure C₆₀ and C₇₀ have been studied by time-resolved degenerate four-wave mixing using femtosecond optical pulses with a wavelength of 633 nm. Large optical nonlinearities were measured for both materials, with χ⁽³⁾ values ≈ 10^-10 esu. The degenerate four-wave mixing signal was monitored as a function of the relative arrival times for the excitation pulses. Along with a long-lived (≈ 100 ps) component to the four-wave mixing decay, response dynamics occurring on both femtosecond and picosecond time scales were observed for both materials.

Original language	English (US)
Pages (from-to)	427-432
Number of pages	6
Journal	Chemical Physics Letters
Volume	196
Issue number	5
DOIs	https://doi.org/10.1016/0009-2614(92)85715-M
State	Published - Aug 21 1992
Externally published	Yes

ASJC Scopus subject areas

General Physics and Astronomy
Physical and Theoretical Chemistry

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10.1016/0009-2614(92)85715-M

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title = "Time-resolved degenerate four-wave mixing in thin films of C60 and C70 using femtosecond optical pulses",

abstract = "Thin films of pure C60 and C70 have been studied by time-resolved degenerate four-wave mixing using femtosecond optical pulses with a wavelength of 633 nm. Large optical nonlinearities were measured for both materials, with χ(3) values ≈ 10-10 esu. The degenerate four-wave mixing signal was monitored as a function of the relative arrival times for the excitation pulses. Along with a long-lived (≈ 100 ps) component to the four-wave mixing decay, response dynamics occurring on both femtosecond and picosecond time scales were observed for both materials.",

author = "Rosker, \{M. J.\} and Marcy, \{H. O.\} and Chang, \{Tallis Y.\} and Khoury, \{J. T.\} and K. Hansen and Whetten, \{R. L.\}",

year = "1992",

month = aug,

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doi = "10.1016/0009-2614(92)85715-M",

language = "English (US)",

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pages = "427--432",

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TY - JOUR

T1 - Time-resolved degenerate four-wave mixing in thin films of C60 and C70 using femtosecond optical pulses

AU - Rosker, M. J.

AU - Marcy, H. O.

AU - Chang, Tallis Y.

AU - Khoury, J. T.

AU - Hansen, K.

AU - Whetten, R. L.

PY - 1992/8/21

Y1 - 1992/8/21

N2 - Thin films of pure C60 and C70 have been studied by time-resolved degenerate four-wave mixing using femtosecond optical pulses with a wavelength of 633 nm. Large optical nonlinearities were measured for both materials, with χ(3) values ≈ 10-10 esu. The degenerate four-wave mixing signal was monitored as a function of the relative arrival times for the excitation pulses. Along with a long-lived (≈ 100 ps) component to the four-wave mixing decay, response dynamics occurring on both femtosecond and picosecond time scales were observed for both materials.

AB - Thin films of pure C60 and C70 have been studied by time-resolved degenerate four-wave mixing using femtosecond optical pulses with a wavelength of 633 nm. Large optical nonlinearities were measured for both materials, with χ(3) values ≈ 10-10 esu. The degenerate four-wave mixing signal was monitored as a function of the relative arrival times for the excitation pulses. Along with a long-lived (≈ 100 ps) component to the four-wave mixing decay, response dynamics occurring on both femtosecond and picosecond time scales were observed for both materials.

UR - https://www.scopus.com/pages/publications/0001351925

UR - https://www.scopus.com/pages/publications/0001351925#tab=citedBy

U2 - 10.1016/0009-2614(92)85715-M

DO - 10.1016/0009-2614(92)85715-M

M3 - Article

AN - SCOPUS:0001351925

SN - 0009-2614

VL - 196

SP - 427

EP - 432

JO - Chemical Physics Letters

JF - Chemical Physics Letters

IS - 5

ER -

Time-resolved degenerate four-wave mixing in thin films of C₆₀ and C₇₀ using femtosecond optical pulses

Abstract

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